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Material Balance Fundamentals

Material balance is the foundation of chemical engineering calculations, based on the law of conservation of mass.

Conservation of Mass

The fundamental principle states that mass can neither be created nor destroyed (excluding nuclear reactions):

Input + Generation = Output + Consumption + Accumulation

For steady-state processes without reaction:

Total Mass In = Total Mass Out

Types of Balances

Overall Material Balance

Accounts for total mass flow across the system boundary:

Σ(min) = Σ(mout)

Component Balance

Tracks individual species through the system:

Σ(min × xi,in) = Σ(mout × xi,out)

Where xi is the mass fraction of component i.

Mass vs Mole Basis

BasisWhen to UseConversion
Mass (kg, lb)Physical processes, mixing, non-reactive systemsn = m / MW
Mole (kmol, mol)Chemical reactions, gas-phase processesm = n × MW

Common Unit Operations

Mixer

Multiple streams combine into one. No reaction occurs.

F1 + F2 = Fout

Splitter

One stream divides into multiple streams with same composition.

Fin = F1 + F2, where xin = x1 = x2

Separator

One stream divides into multiple streams with different compositions.

Fin = F1 + F2, where xin ≠ x1 ≠ x2

Reactor

Chemical reaction occurs. Use extent of reaction (ξ) or conversion (X).

ni,out = ni,in + νi × ξ

Reactive Systems

For systems with chemical reactions, the balance includes generation and consumption terms:

Extent of Reaction (ξ)

For reaction: aA + bB → cC + dD

nA,out = nA,in - a×ξ

nC,out = nC,in + c×ξ

Conversion (X)

X = (nA,in - nA,out) / nA,in

Degrees of Freedom Analysis

Before solving, check if the problem is properly specified:

DOF = Unknowns - Independent Equations

  • DOF = 0: Exactly determined, unique solution exists
  • DOF > 0: Under-specified, need more information
  • DOF < 0: Over-specified, check for inconsistencies

Solving Procedure

  1. Draw and label the flowsheet
  2. Choose a basis (e.g., 100 kg/h or 1 kmol)
  3. Identify all streams and components
  4. Write overall material balance
  5. Write component balances
  6. Perform degrees of freedom analysis
  7. Solve the system of equations
  8. Check results (sum of fractions = 1, all values positive)

References

  • Felder, R.M. and Rousseau, R.W. (2005). Elementary Principles of Chemical Processes. Wiley.
  • Himmelblau, D.M. and Riggs, J.B. (2012). Basic Principles and Calculations in Chemical Engineering. Prentice Hall.
  • Perry, R.H. and Green, D.W. (2008). Perry's Chemical Engineers' Handbook. McGraw-Hill.